This study reports the development of a high-performance supercapacitor utilizing a templated carbon electrode (graphene mesosponge; GMS) and a novel ionogel electrolyte. By integrating an ionic liquid ([EMIM]+[HSO4]-) within a PVA/GMS polymer matrix, the device achieves enhanced electrochemical stability and ion mobility. Electrochemical characterization via CV, EIS, and GCD demonstrates superior capacitive behaviour and reduced internal resistance (IR drop). The results were supported by computational models that confirms that GMS's unique structure enhances ion accessibility and interaction and the ionogel enables efficient charge storage, offering a promising strategy for flexible and robust energy storage applications.
- Amrita Jain
- Daniel Moreno-Rodríguez
- Eva Scholtzova